TY - JOUR
T1 - Acoustic Manipulation of Deterministic Quantum Emitters in WSe2
AU - Mohajerani, Seyed Sepehr
AU - Noual, Adnane
AU - Ma, Yichen
AU - Koneru, Dheeraj
AU - Kumar, Pankaj
AU - Tang, Yunong
AU - Xiao, Licheng
AU - Chen, Siwei
AU - Liu, Yuxing
AU - Hone, James
AU - Yang, Eui Hyeok
AU - Strauf, Stefan
N1 - Publisher Copyright:
© 2025 American Chemical Society
PY - 2025/7/22
Y1 - 2025/7/22
N2 - Surface acoustic waves (SAWs) have recently emerged as a powerful tool for controlling excitonic states in two-dimensional (2D) transition metal dichalcogenides, enabling dynamic energy modulation and transport of carriers over micron-scale distances. Yet, the use of SAWs to realize direct, high-speed manipulation of site-controlled quantum emitters (QEs) in 2D materials remains largely unexplored. Here, we show acoustic manipulation of deterministic, strain-induced QEs in monolayer WSe2by interfacing them with SAWs on a lithium niobate substrate. Using gold nanocube stressors to precisely engineer local strain, we overcome the stochastic nature of defect-based QEs. Upon SAW excitation, these deterministic QEs exhibit an energy shift of up to 0.58 meV at tuning bandwidth up to 8 MHz, enabling half-GHz optical modulation speed despite residing 210 nm above the SAW-carrying substrate. Power-dependent experiments reveal a nonlinear response regime of the SAW-driven nanocube stressor for RF excitation near the energetically lowest-lying flexural mode, highlighting the acousto-optical transduction in our device. Our findings provide a robust, scalable approach for fast, dynamic tuning of single photons with strongly suppressed spectral diffusion and may offer opportunities for nanoscale quantum sensors capable of mapping out acoustic fields with subwavelength spatial resolution on a chip.
AB - Surface acoustic waves (SAWs) have recently emerged as a powerful tool for controlling excitonic states in two-dimensional (2D) transition metal dichalcogenides, enabling dynamic energy modulation and transport of carriers over micron-scale distances. Yet, the use of SAWs to realize direct, high-speed manipulation of site-controlled quantum emitters (QEs) in 2D materials remains largely unexplored. Here, we show acoustic manipulation of deterministic, strain-induced QEs in monolayer WSe2by interfacing them with SAWs on a lithium niobate substrate. Using gold nanocube stressors to precisely engineer local strain, we overcome the stochastic nature of defect-based QEs. Upon SAW excitation, these deterministic QEs exhibit an energy shift of up to 0.58 meV at tuning bandwidth up to 8 MHz, enabling half-GHz optical modulation speed despite residing 210 nm above the SAW-carrying substrate. Power-dependent experiments reveal a nonlinear response regime of the SAW-driven nanocube stressor for RF excitation near the energetically lowest-lying flexural mode, highlighting the acousto-optical transduction in our device. Our findings provide a robust, scalable approach for fast, dynamic tuning of single photons with strongly suppressed spectral diffusion and may offer opportunities for nanoscale quantum sensors capable of mapping out acoustic fields with subwavelength spatial resolution on a chip.
KW - nonlinear response
KW - optomechanics
KW - quantum emitters
KW - surface acoustic waves
KW - tungsten diselenide
UR - https://www.scopus.com/pages/publications/105010199261
UR - https://www.scopus.com/pages/publications/105010199261#tab=citedBy
U2 - 10.1021/acsnano.5c04710
DO - 10.1021/acsnano.5c04710
M3 - Article
C2 - 40631535
AN - SCOPUS:105010199261
SN - 1936-0851
VL - 19
SP - 25851
EP - 25859
JO - ACS Nano
JF - ACS Nano
IS - 28
ER -