TY - JOUR
T1 - Pulse function for control of the coherent excitation in stimulated raman spectroscopy
AU - Malinovskaya, S. A.
PY - 2005/4/5
Y1 - 2005/4/5
N2 - A selective excitation of closely spaced Raman transitions using femtosecond pulse shaping is studied within a semiclassical approach. An analytical pulse function is proposed having duration T that selectively excites one of two transitions separated by a frequency interval less than 1/T. It is shown that, for intense fields, both the field amplitude and pulse frequency spectrum have to be carefully chosen to achieve the control of excitations.
AB - A selective excitation of closely spaced Raman transitions using femtosecond pulse shaping is studied within a semiclassical approach. An analytical pulse function is proposed having duration T that selectively excites one of two transitions separated by a frequency interval less than 1/T. It is shown that, for intense fields, both the field amplitude and pulse frequency spectrum have to be carefully chosen to achieve the control of excitations.
KW - Coherent states
KW - Femtosecond pulse control
KW - Mode selective excitation
KW - Stimulated raman scattering
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U2 - 10.1002/qua.20393
DO - 10.1002/qua.20393
M3 - Article
AN - SCOPUS:15944387960
SN - 0020-7608
VL - 102
SP - 313
EP - 317
JO - International Journal of Quantum Chemistry
JF - International Journal of Quantum Chemistry
IS - 3
ER -