STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS

Anthony Palumbo; Chenguang Zhao; Hongjun Wang; Kalle Levon; Eui Hyeok Yang

STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS

Anthony Palumbo, Chenguang Zhao, Hongjun Wang, Kalle Levon, Eui Hyeok Yang

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

This paper presents a stretchable glucose sensor composed of dodecylbenzenesulfonate-doped polypyrrole (PPy(DBS))-coated vertically aligned carbon nanotube (VACNT) forests partially embedded in a polydimethylsiloxane (PDMS) substrate. VACNTs are grown via chemical vapor deposition (CVD) and transferred onto partially cured PDMS. A conformal PPy(DBS) layer is electropolymerized on the nanotubes to create PPy(DBS)-coated VACNTs. Next, dip-coating is performed in glucose oxidase (GOx) solution to immobilize GOx with glutaraldehyde (GA) as a crosslinking agent onto the PPy(DBS) surface. The PDMS/CNT/PPy(DBS)/GOx is exposed to varying glucose concentrations to measure its amperometric response. The sensor exhibits a sensitivity of 10 mA cm^-2 M^-1, a linear range of 0.1 mM to 12 mM, and a response time shorter than 5 seconds. Strain is applied to the sensor device, demonstrating its stable sensing function up to 75% strain and with coefficients of determination large than 0.975.

Original language	English
Title of host publication	2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022
Editors	Reza Ghodssi, Jenna F. Chan
Pages	324-327
Number of pages	4
ISBN (Electronic)	9781940470047
State	Published - 2022
Event	2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022 - Hilton Head, United States Duration: 5 Jun 2022 → 9 Jun 2022

Publication series

Name	2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022

Conference

Conference	2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022
Country/Territory	United States
City	Hilton Head
Period	5/06/22 → 9/06/22

Keywords

Flexible electrode
carbon nanotubes
electrochemical sensing
glucose sensor
polypyrrole

Cite this

Palumbo, A., Zhao, C., Wang, H., Levon, K., & Yang, E. H. (2022). STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS. In R. Ghodssi, & J. F. Chan (Eds.), 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022 (pp. 324-327). (2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022).

Palumbo, Anthony ; Zhao, Chenguang ; Wang, Hongjun et al. / STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS. 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022. editor / Reza Ghodssi ; Jenna F. Chan. 2022. pp. 324-327 (2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022).

@inproceedings{3a3efe379ee94663b51e6be4c7946eca,

title = "STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS",

abstract = "This paper presents a stretchable glucose sensor composed of dodecylbenzenesulfonate-doped polypyrrole (PPy(DBS))-coated vertically aligned carbon nanotube (VACNT) forests partially embedded in a polydimethylsiloxane (PDMS) substrate. VACNTs are grown via chemical vapor deposition (CVD) and transferred onto partially cured PDMS. A conformal PPy(DBS) layer is electropolymerized on the nanotubes to create PPy(DBS)-coated VACNTs. Next, dip-coating is performed in glucose oxidase (GOx) solution to immobilize GOx with glutaraldehyde (GA) as a crosslinking agent onto the PPy(DBS) surface. The PDMS/CNT/PPy(DBS)/GOx is exposed to varying glucose concentrations to measure its amperometric response. The sensor exhibits a sensitivity of 10 mA cm-2 M-1, a linear range of 0.1 mM to 12 mM, and a response time shorter than 5 seconds. Strain is applied to the sensor device, demonstrating its stable sensing function up to 75% strain and with coefficients of determination large than 0.975.",

keywords = "Flexible electrode, carbon nanotubes, electrochemical sensing, glucose sensor, polypyrrole",

author = "Anthony Palumbo and Chenguang Zhao and Hongjun Wang and Kalle Levon and Yang, {Eui Hyeok}",

note = "Publisher Copyright: {\textcopyright} 2022 TRF.; 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022 ; Conference date: 05-06-2022 Through 09-06-2022",

year = "2022",

language = "English",

series = "2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022",

pages = "324--327",

editor = "Reza Ghodssi and Chan, {Jenna F.}",

booktitle = "2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022",

}

Palumbo, A, Zhao, C, Wang, H, Levon, K & Yang, EH 2022, STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS. in R Ghodssi & JF Chan (eds), 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022. 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022, pp. 324-327, 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022, Hilton Head, United States, 5/06/22.

STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS. / Palumbo, Anthony; Zhao, Chenguang; Wang, Hongjun et al.
2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022. ed. / Reza Ghodssi; Jenna F. Chan. 2022. p. 324-327 (2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

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T1 - STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS

AU - Palumbo, Anthony

AU - Zhao, Chenguang

AU - Wang, Hongjun

AU - Levon, Kalle

AU - Yang, Eui Hyeok

PY - 2022

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N2 - This paper presents a stretchable glucose sensor composed of dodecylbenzenesulfonate-doped polypyrrole (PPy(DBS))-coated vertically aligned carbon nanotube (VACNT) forests partially embedded in a polydimethylsiloxane (PDMS) substrate. VACNTs are grown via chemical vapor deposition (CVD) and transferred onto partially cured PDMS. A conformal PPy(DBS) layer is electropolymerized on the nanotubes to create PPy(DBS)-coated VACNTs. Next, dip-coating is performed in glucose oxidase (GOx) solution to immobilize GOx with glutaraldehyde (GA) as a crosslinking agent onto the PPy(DBS) surface. The PDMS/CNT/PPy(DBS)/GOx is exposed to varying glucose concentrations to measure its amperometric response. The sensor exhibits a sensitivity of 10 mA cm-2 M-1, a linear range of 0.1 mM to 12 mM, and a response time shorter than 5 seconds. Strain is applied to the sensor device, demonstrating its stable sensing function up to 75% strain and with coefficients of determination large than 0.975.

AB - This paper presents a stretchable glucose sensor composed of dodecylbenzenesulfonate-doped polypyrrole (PPy(DBS))-coated vertically aligned carbon nanotube (VACNT) forests partially embedded in a polydimethylsiloxane (PDMS) substrate. VACNTs are grown via chemical vapor deposition (CVD) and transferred onto partially cured PDMS. A conformal PPy(DBS) layer is electropolymerized on the nanotubes to create PPy(DBS)-coated VACNTs. Next, dip-coating is performed in glucose oxidase (GOx) solution to immobilize GOx with glutaraldehyde (GA) as a crosslinking agent onto the PPy(DBS) surface. The PDMS/CNT/PPy(DBS)/GOx is exposed to varying glucose concentrations to measure its amperometric response. The sensor exhibits a sensitivity of 10 mA cm-2 M-1, a linear range of 0.1 mM to 12 mM, and a response time shorter than 5 seconds. Strain is applied to the sensor device, demonstrating its stable sensing function up to 75% strain and with coefficients of determination large than 0.975.

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KW - polypyrrole

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M3 - Conference contribution

AN - SCOPUS:85172664861

T3 - 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022

SP - 324

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BT - 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022

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Y2 - 5 June 2022 through 9 June 2022

ER -

Palumbo A, Zhao C, Wang H, Levon K, Yang EH. STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS. In Ghodssi R, Chan JF, editors, 2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022. 2022. p. 324-327. (2022 Solid-State Sensors, Actuators and Microsystems Workshop, Hilton Head 2022).

STRETCHABLE GLUCOSE SENSOR VIA CONJUGATED POLYMER CONFORMALLY-COATED CNT ELECTRODES PARTIALLY EMBEDDED IN PDMS

Abstract

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